Can I bulk-remove users from Opportunities at the Organization level?

InitLive is now Bloomerang Volunteer—a new name, a new look, and a new integration. Bloomerang Volunteer works just like InitLive. You can do everything you always do, and in the same way. 

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Yes, Managers can bulk-remove users from Opportunities using the Organization Staff List. After selecting all the users that you want to remove from an Opportunity, Managers can use the Take Action dropdown to select the Opportunity they want the staff/volunteers removed from.